With the advent of self-healing (SH) materials a new vision of material science had been accomplished, together with the exploitation of specific chemical and physical principles. Thus e.g. fast crosslinking and crack-repair after damage has been optimized via encapsulation and embedding of reactive components;  the application of supramolecular bonds has enabled multiple self-healing taking into account the relevant timescales of self-healing. The current presentation addresses principles of self-healing polymers taking place at the site of damage specifically via stress-induced chemical reactions, in particular "click"-based chemistries to induce self-healing responses via force-induced healing. By introducing supramolecular healing principles mechanically stronger materials are obtained, displaying multiple healing-cycles together with eg. graphene-based nanofillers bearing attached catalytic systems.
Acknowledgements. Financial support from the DFG (project Bi 1337-1/8) within the framework of SPP 1568 (Design and Generic Principles of Self-Healing Polymers) and the EU-project IASS (within EU-FP7) are gratefully acknowledged.
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